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Ynamide Preactivation Allows a Regio- and Stereoselective Synthesis of alpha,beta-Disubstituted Enamides
A novel ynamide preactivation strategy enables the use of otherwise incompatible reagents and allows preparation of alpha,beta-disubstituted enamides with high regio- and stereoselectivity. Mechanistic analysis reveals the intermediacy of a triflate-bound intermediate as a solution-stable, effective keteniminium reservoir, whilst still allowing subsequent addition of organometallic reagents.
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Oxazolidine – Wikipedia,
Oxazolidine | C3H331NO – PubChem