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Directed, regiocontrolled hydroamination of unactivated alkenes via protodepalladation
A directed, regiocontrolled hydroamination of unactivated terminal and internal alkenes is reported. The reaction is catalyzed by palladium(II) acetate and is compatible with a variety of nitrogen nucleophiles. A removable bidentate directing group is used to control the regiochemistry, prevent beta-hydride elimination, and stabilize the nucleopalladated intermediate, facilitating a protodepalladation event. This method affords highly functionalized amino acids in good yields with high regioselectivity.
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Reference£º
Oxazolidine – Wikipedia,
Oxazolidine | C3H580NO – PubChem